To make something form into crystals
I crystallized the copper sulphate by slowly cooling a saturated solution.
To assume a crystalline form
The copper sulphate crystallized from solution.
To give something a definite or precise form
After some thought, I crystallized my ideas for the paper.
To take a definite form
My ideas crystallized overnight.
To coat something with crystals, especially with sugar
We crystallized the fruit by coating in sugar.